Introducing tin to develop ternary metal oxides with excellent hydrothermal stability for NH3 selective catalytic reduction of NOx

RCEES OpenIR > 水污染控制实验室

	Introducing tin to develop ternary metal oxides with excellent hydrothermal stability for NH3 selective catalytic reduction of NOx
	Liu, Jingjing; He, Guangzhi ; Shan, Wenpo ; Yu, Yunbo ; Huo, Yanlong ; Zhang, Yan ; Wang, Meng ; Yu, Rong ; Liu, Shengsheng ; He, Hong
	2021-08-15
Source Publication	APPLIED CATALYSIS B-ENVIRONMENTAL
ISSN	0926-3373
Volume	291 Pages:-
Abstract	Thermal stability is crucial for the practical application of heterogeneous catalysts. In particular, the development of catalysts with excellent hydrothermal stability remains a big challenge for diesel exhaust after-treatment technologies. Here, we synthesized a Ce1W0.24Sn2Ox catalyst with high hydrothermal stability for the NOx removal from diesel engines. The catalyst shows >90 % NOx conversion at 300 550 degrees C even after an extreme aging treatment at 1000 degrees C, with much better hydrothermal stability than the Ce1W0.24Ox catalyst and the commercial catalysts such as Cu-SSZ-13 and V2O5-WO3/TiO2. The experimental and theoretical results reveal that the SnO2-related particles modified by W and Ce species show outstanding sintering resistance at high temperature, which provides sufficient Ce-W active phase for the catalytic reaction. This study may provide new opportunities for the application of metal oxide catalysts for diesel engine NOx emission control and a new idea for the development of catalysts with high thermal stability.
Department	水污染控制实验室
Keyword	Heterogeneous catalysis NOx removal Hydrothermal stability Anti-sintering SnO2
WOS Research Area	Chemistry, Physical ; Engineering, Environmental ; Engineering, Chemical
Document Type	期刊论文
Identifier	https://ir.rcees.ac.cn/handle/311016/46049
Collection	水污染控制实验室
Affiliation	1.Chinese Acad Sci, Res Ctr Ecoenvironm Sci, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100085, Peoples R China 2.Chinese Acad Sci, Ctr Excellence Reg Atmospher Environm, Inst Urban Environm, Xiamen 361021, Peoples R China 3.Tsinghua Univ, Natl Ctr Electron Microscopy Beijing, Sch Mat Sci & Engn, Key Lab Adv Mat,Minist Educ China,State Key Lab N, Beijing 4.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
Recommended Citation GB/T 7714	Liu, Jingjing,He, Guangzhi,Shan, Wenpo,et al. Introducing tin to develop ternary metal oxides with excellent hydrothermal stability for NH3 selective catalytic reduction of NOx[J]. APPLIED CATALYSIS B-ENVIRONMENTAL,2021,291:-.
APA	Liu, Jingjing.,He, Guangzhi.,Shan, Wenpo.,Yu, Yunbo.,Huo, Yanlong.,...&He, Hong.(2021).Introducing tin to develop ternary metal oxides with excellent hydrothermal stability for NH3 selective catalytic reduction of NOx.APPLIED CATALYSIS B-ENVIRONMENTAL,291,-.
MLA	Liu, Jingjing,et al."Introducing tin to develop ternary metal oxides with excellent hydrothermal stability for NH3 selective catalytic reduction of NOx".APPLIED CATALYSIS B-ENVIRONMENTAL 291(2021):-.

Files in This Item:
File Name/Size	DocType	Version	Access	License
Introducing tin to d（6353KB）	期刊论文	出版稿	开放获取	CC BY-NC-SA	View Application Full Text

File name:	Introducing tin to develop ternary metal oxides with excellent hydrothermal stability for NH3 selective catalytic reduction of NOx.pdf
Format:	Adobe PDF

If you have any objections to this item, please fill out the form below and the administrator will contact you as soon as possible.
Content:
Email：	*
Institution:
Verification Code:	Refresh

Any comments and suggestions are welcomed.
Title:	*
Content:
Email：	*
Verification Code:	Refresh

水污染控制实验室知识库