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Occurrence, distribution and ecological risk assessment of polycyclic aromatic hydrocarbons and their derivatives in the effluents of wastewater treatment plants
Liu, Quanzhen; Xu, Xiong; Lin, Lihua; Wang, Donghong
2021-10-01
Source PublicationSCIENCE OF THE TOTAL ENVIRONMENT
ISSN0048-9697
Volume789Pages:-
AbstractIn this study, we investigated the concentration distribution of parent polycyclic aromatic hydrocarbons (PAHs) and their derivatives in the effluents of 5 municipal wastewater treatment plants (WWTPs) in Beijing, China for eight months. We first identified the coexistence of PAHs, chlorinated PAHs (CI-PAHs), brominated PAHs (Br-PAHs) and oxygenated PAHs (OPAHs) in the effluents of WWTPs. Three CI-PAHs and 7 Br-PAHs were first found. The total concentrations of PAHs, Cl-PAHs, Br-PAHs and OPAHs ranged from 8.99-88.38, n.d.-5.70, n.d.-13.11 ng L-1 and 15.47-106.92 ng L-1, respectively. In terms of temporal distributions, the total concentrations of PAHs and OPAHs presented a decreasing trend from April to November and the total concentrations of Cl-PAHs and Br-PAHs fluctuated at lower levels. These results indicated that these compounds will be long-term discharged into the receiving river. In addition, Cl-PAHs, Br-PAHs and OPAHs were likely generated by transformations occurring during chlori nation disinfection. For ecological risk assessment, risk quotients of 6 compounds, indeno[1,2,3-cd] pyrene, benzo[g,h,i]perylene, dibenz[a,h]anthracene, 6-bromobenzo[a]pyrene, 1,8-dibromopyrene and 1,6-dibromopyrene, were thought to indicate high ecological risk (fish). Furthermore, Cl-PAHs, Br-PAHs and OPAHs in the effluents of WWTPs can cause more serious environmental hazards than the corresponding PAHs. (C) 2021 Elsevier B.V. All rights reserved.
Department中国科学院饮用水科学与技术重点实验室
KeywordWastewater treatment plants Effluent Disinfection by-products Temporal distribution Ecological risk
WOS Research AreaEnvironmental Sciences
Document Type期刊论文
Identifierhttps://ir.rcees.ac.cn/handle/311016/46244
Collection中国科学院饮用水科学与技术重点实验室
Affiliation1.Chinese Acad Sci, Res Ctr Eco Environm Sci, Key Lab Drinking Water Sci & Technol, Beijing 100085, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
Recommended Citation
GB/T 7714
Liu, Quanzhen,Xu, Xiong,Lin, Lihua,et al. Occurrence, distribution and ecological risk assessment of polycyclic aromatic hydrocarbons and their derivatives in the effluents of wastewater treatment plants[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2021,789:-.
APA Liu, Quanzhen,Xu, Xiong,Lin, Lihua,&Wang, Donghong.(2021).Occurrence, distribution and ecological risk assessment of polycyclic aromatic hydrocarbons and their derivatives in the effluents of wastewater treatment plants.SCIENCE OF THE TOTAL ENVIRONMENT,789,-.
MLA Liu, Quanzhen,et al."Occurrence, distribution and ecological risk assessment of polycyclic aromatic hydrocarbons and their derivatives in the effluents of wastewater treatment plants".SCIENCE OF THE TOTAL ENVIRONMENT 789(2021):-.
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