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Microwave-assisted continuous flow phytosynthesis of silver nanoparticle/reduced graphene oxide composites and related visible light catalytic performance
Wang, Houyu; Yuan, Chun-Gang; Liu, Chenchen; Duan, Xuelei; Guo, Qi; Shen, Yiwen; Liu, Jingfu; Chen, Yongsheng
2022-05
Source PublicationJOURNAL OF ENVIRONMENTAL SCIENCES
ISSN1001-0742
Volume115Issue:0Pages:286-293
AbstractThe creation of an environmentally friendly synthesis method for silver nanomaterials (AgNPs) is an urgent concern for sustainable nanotechnology development. In the present study, a novel straightforward and green method for the preparation of silver nanoparticle/reduced graphene oxide (AgNP/rGO) composites was successfully developed through the combination of phytosynthesis, continuous flow synthesis and microwave-assistance. Oriental persimmon (Diospyros kaki Thunb.) extracts were used as both plant reducing and capping agents for fast online synthesis of AgNP/rGO composites. The experimental parameters were optimized and the morphologies of the prepared materials were investigated. The characterization results reveal that spherical AgNPs were quickly synthesized and uniformly dispersed on rGO sheets using the proposed online system. Fourier transform infrared spectroscopy analysis confirmed that phenols, flavonoids, and other substances in the plant extracts played a decisive role in the synthesis of AgNP/rGO composites. Using sodium borohydride (NaBH4) degradation of p-nitrophenol (4-NP) as a model, the catalytic activity of the prepared AgNP/rGO materials was evaluated. The complete degradation of 4-NP was achieved within 12 min through the use of AgNP/rGO materials, and the composite had a much better catalytic activity than the bare AgNPs and rGO had. Compared with the conventional chemical method, our online method is facile, fast, cost-efficient, and environmentally friendly. (C) 2021 The Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences. Published by Elsevier B.V.
Department环境化学与生态毒理学国家重点实验室 ; 环境化学与生态毒理学国家重点实验室
KeywordGREEN SYNTHESIS QUANTIFICATION REDUCTION EXTRACTS
Document Type期刊论文
Identifierhttps://ir.rcees.ac.cn/handle/311016/47575
Collection环境化学与生态毒理学国家重点实验室
Affiliation1.North China Elect Power Univ, Dept Environm Sci & Engn, Hebei Key Lab Power Plant Flue Gas Multipollutant, Baoding 071000, Peoples R China
2.North China Elect Power Univ, Wetland Res Ctr Baiyangdian Lake, Baoding 071000, Peoples R China
3.Chinese Acad Sci, Res Ctr Ecoenvironm Sci, State Key Lab Environm Chem & Ecotoxicol, Beijing 100085, Peoples R China
4.Georgia Inst Technol, Sch Civil & Environm Engn, Atlanta, GA 30332 USA
Recommended Citation
GB/T 7714
Wang, Houyu,Yuan, Chun-Gang,Liu, Chenchen,et al. Microwave-assisted continuous flow phytosynthesis of silver nanoparticle/reduced graphene oxide composites and related visible light catalytic performance[J]. JOURNAL OF ENVIRONMENTAL SCIENCES,2022,115(0):286-293.
APA Wang, Houyu.,Yuan, Chun-Gang.,Liu, Chenchen.,Duan, Xuelei.,Guo, Qi.,...&Chen, Yongsheng.(2022).Microwave-assisted continuous flow phytosynthesis of silver nanoparticle/reduced graphene oxide composites and related visible light catalytic performance.JOURNAL OF ENVIRONMENTAL SCIENCES,115(0),286-293.
MLA Wang, Houyu,et al."Microwave-assisted continuous flow phytosynthesis of silver nanoparticle/reduced graphene oxide composites and related visible light catalytic performance".JOURNAL OF ENVIRONMENTAL SCIENCES 115.0(2022):286-293.
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