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Bicomponent Cocatalyst Decoration on Flux-assisted CaTaO2N Single Crystals for Photocatalytic CO2 Reduction under Visible Light
Zhou, Hanghang; Luo, Ying; Xu, Jun; Deng, Lidan; Wang, Zheng; He, Hong
2022
Source PublicationCHEMISTRY-A EUROPEAN JOURNAL
ISSN0947-6539
Pages1-8
AbstractCubic-like CaTaO2N photocatalysts with high crystallinity and uniform particle size were successfully prepared by the flux-assisted nitridation method. The growth of CaTaO2N single crystals under different synthesis conditions was systematically investigated to understand the effects of the crystallinity and optical property on photocatalytic performance of CO2 reduction. Moreover, the modification of CaTaO2N single crystals with core-shell Ni-Ag bicomponent cocatalyst by two-step decoration process gave a 2.4 times higher amount of CO evolution than the deposition of sole Ag cocatalyst, because of the synergistic effects of bicomponent cocatalyst on the interfacial electron transfer and surface catalytic process. This study provides a valuable way to construct high-crystalline photocatalysts with effective bicomponent cocatalyst for visible-light-driven CO2 reduction with H2O.
Department大气环境与污染控制实验室
Keywordbicomponent cocatalyst CaTaO2N crystal CO2 reduction flux visible light
Document Type期刊论文
Identifierhttps://ir.rcees.ac.cn/handle/311016/48445
Collection大气环境与污染控制实验室
Affiliation1.Chinese Academy of Sciences
2.Research Center for Eco-Environmental Sciences (RCEES)
3.University of Chinese Academy of Sciences, CAS
4.Huazhong University of Science & Technology
Recommended Citation
GB/T 7714
Zhou, Hanghang,Luo, Ying,Xu, Jun,et al. Bicomponent Cocatalyst Decoration on Flux-assisted CaTaO2N Single Crystals for Photocatalytic CO2 Reduction under Visible Light[J]. CHEMISTRY-A EUROPEAN JOURNAL,2022:1-8.
APA Zhou, Hanghang,Luo, Ying,Xu, Jun,Deng, Lidan,Wang, Zheng,&He, Hong.(2022).Bicomponent Cocatalyst Decoration on Flux-assisted CaTaO2N Single Crystals for Photocatalytic CO2 Reduction under Visible Light.CHEMISTRY-A EUROPEAN JOURNAL,1-8.
MLA Zhou, Hanghang,et al."Bicomponent Cocatalyst Decoration on Flux-assisted CaTaO2N Single Crystals for Photocatalytic CO2 Reduction under Visible Light".CHEMISTRY-A EUROPEAN JOURNAL (2022):1-8.
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